I'd do a really glossy sheer red lip and for the eyes, I'd do really dramatic fake lashes with a sparkly sheer white-ish look on the "Angel" side. On the "Devil" side, I'd do a neutral lid but with a wicked cat eye in black liner, or I'd do on that eye in red if you can carry off red on the eyes (I can't!).
Of course, I wouldn't mind walking around with two mismatched eyes. If you do, just do the really glossy sheer red lip and one or the other of the eye looks.